A donor–π–σ–acceptor strategy in porous polymers for suppression of carrier recombination: boosting photoredox in a Csp2–N radical cross-coupling reaction

Green Chem., 2025, Advance Article
DOI: 10.1039/D5GC02546J, Paper

Jinyang Lu, Lingjuan Zhang, Nan Zhang, Xueying Song, Qi Gao, Jincong Yuan, Xian-Ming Zhang
Incorporating σ linker between the D–π–A heterojunction suppresses photogenerated carrier recombination. ETTA-σ-Im exhibits highly catalytic performance in photooxidative CDC amidation, while facilitating photoreductive O₂ to H₂O₂ production.
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