Regulating the hydrophobic microenvironment of SnS2 to facilitate the interfacial CO2/H2O ratio towards pH-universal electrocatalytic CO2 reduction

Green Chem., 2025, Advance Article
DOI: 10.1039/D5GC00635J, Paper

Zhiwei Dong, Yaling Jia, Zeyu Wang, Antony Rajendran, Wen-Ying Li
A hydrophobic microenvironment near SnS₂ was constructed using polyvinylidene fluoride modification, which could increase the CO₂ concentration around SnS₂ surface. This strategy could enhance catalytic performance of SnS₂ across a wide pH range.
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