Green direct recycling of spent LiFePO4 via electronic structure reconstruction and reinforced Fe–O d–p orbital hybridization for enhanced energy storage performance

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Green Chem., 2026, Advance Article
DOI: 10.1039/D5GC06175J, Paper
Zonghao Xu, Zongyu Guan, Yan Song, Xiran Zhao, Yaodong Yuan, Zhipeng Yan, Junhang Tian, Xueyi Sun, Biwei Xiao, Weidong Zhuang
A mild, low-energy LiI-assisted route regenerates spent LFP by replenishing Li, eliminating Fe–Li antisite defects and rebuilding Li+ channels, while strengthened Fe–O d–p hybridization stabilizes the framework for sustainable cathode recycling.
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