Closed-loop electro-upcycling of PET waste into formate and hydrogen via self-supported NiCo2O4 spinel arrays

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Green Chem., 2025, Advance Article
DOI: 10.1039/D5GC01993A, Paper
Mingkun Jiang, Yang Yang, Yujie Wang, Yajie Wang, Marina Ratova, Dan Wu
NiCo2O4 electrocatalyst upcycles PET to formate (96.7% FE) and H2 at 400 mA cm−2, giving $774.56 per ton PET. Ni–Co sites cleave C–C bonds while limiting overoxidation, enabling sustainable plastic valorization.
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